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Excitation of coherent phonons has the potential to dramatically alter the electronic structure of Dirac and Weyl semimetals, enabling sub-picosecond control of their optical and electronic properties. The Dirac semimetal SrMnSb2 is a candidate for such control, with a coherent-phonon mode that is predicted to close and reopen a gap at the Dirac node. Here, through a series of ultrafast pump-probe experiments, we establish suitable samples and conditions for driving the coherent phonon to high amplitude and attempting to observe the gap’s closure. Films of SrMnSb2 grown by molecular-beam epitaxy are shown to have phononic properties matching those of bulk crystals. We find that the phonon can be strongly excited by pump pulses with wavelength near 1500 nm, which will excite a 30-nm film almost uniformly and will penetrate the arsenic capping layers that protect the films. We find that samples withstand pump pulses of fluence up to 20 mJ/cm2, and we demonstrate the potential for sequences of pulses to amplify the oscillation while suppressing other phonon modes. Armed with our new knowledge of the conditions for exciting the desired coherent phonon, future experiments will be well prepared to measure its motion and to observe phononic control of the Dirac-point gap. 

We present a novel, to the best of knowledge, time-resolved, optical pump/NIR supercontinuum probe spectrometer suitable for oscillators. A NIR supercontinuum probe spectrum (850–1250 nm) is generated in a photonic crystal fiber, dispersed across a digital micromirror device (DMD), and then raster scanned into a single element detector at a 5 Hz rate. Dual modulation of pump and probe beams at disparate frequencies permits simultaneous measurement of both the bare reflectanceRand its photoinduced change ΔRthrough lock-in detection, allowing for continuously self-normalized measurement of ΔR/R. Example data are presented on a germanium wafer sample that demonstrate for signals of order ΔR/R ∼ 10⁻³, a 2.87 nm spectral resolution and $\lesssim <\#comment/>400$ fs temporal resolution pre-recompression, and comparable sensitivity to standard time-resolved, amplifier-based pump–probe techniques. 

We report on an ultralow probe-power transient grating apparatus with probing based on a laser diode pulser, a digital delay generator, and a data acquisition card. The electronic triggering of the diode pulser permits stroboscopic measurement of arbitrarily slow laser-induced dynamics using pulses of probe light with average power $\sim <\#comment/>5\mathrm{n}\mathrm{W}$, significantly lower than what is currently used by continuous wave measurement. The proposed method also allows for flexibility in selection of the probe wavelength limited only by availability of low threshold current laser diodes. Examples of impulsive stimulated thermal scattering measurements are presented on liquid isopropanol, single crystal solid ${\mathrm{C}\mathrm{r}\mathrm{C}\mathrm{l}}_3$, and a thin film of Cu vapor deposited on a Si substrate, demonstrating the flexibility of the technique.